有序介孔材料在生物医药领域中的应用

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:200512,:200623(No.GC04C208)33e2mail:wangy-msn@hotmail.com333(150001),,,,:TB383;Q819:A:10052281X(2006)1021345207OrderedMesoporousMaterialsforBiologyandMedicineWangYan33ZhengXuhanJiangZhaohua(DepartmentofAppliedChemistry,HarbinInstituteofTechnology,Harbin150001,China)AbstractInthispaperthemainpropertiesoforderedmesoporousmaterialsarebrieflydescribedandtheirvariousapplicationsintheareasofbiologyandmedicinearereviewedindetails,suchasenzymeimmobilization,biosensors,drugdelivery,bioactivematerialsandseparationsofbiologicalmolecules.Thedevelopmentandperformancesofthematerialsfortheseapplicationsarediscussed.Moreover,expectationofimprovementsinmaterialsandoutlookoftheirpotentialapplicationsareproposed.Keywordsmesoporousmaterials;enzymeimmobilization;biosensors;drugdelivery;bioactivematerials11992,Mobil,1161010nmM41S,[1,2],,[37],2,[3];,,11810200610PROGRESSINCHEMISTRYVol.18No.10Oct.,20061Table1Samplesofmesoporousmaterialsandtheirstructuralcharactersmaterialphaseporechannelporediameter(nm)MCM241hexagonaltwo2dimensional(straight)210MCM248cubicthree2dimensional(intercrossed)24MCM250lamellartwo2dimensional(straight)1020FSM216hexagonaltwo2dimensional(straight)4HMShexagonalshort2rangeordered210MSU2nhexagonalwormholelike215SBA21cubicthree2dimensional(cagelike)23SBA215hexagonaltwo2dimensional(straight)530SBA216cubicthree2dimensional(intercrossed)53033.1110010nm,250nm,2[810],,2,;,2,;,1996,Balkus[11]C40!MCM241,(48!),MCM241MCM248SBA215[1216],,,,CMCM248[17],,[18,19],[20][2144],,,,,,,Takahashi[21]MCM241FSM216,SBA215,,,,MCM241FSM216SBA215,,MCM241FSM216SBA215,,,,[2729],Zhao,[3032],,SBA215[30],FDU212[32],149nm,6431181:a),b);[32]Fig.1Schematicdrawingofthecavityandentranceofacagelikemesoporousmaterialwithsimilarcavitysizesbutdifferententrancesizes:(a)smallentrance;(b)largeentrance.Thediffusionratesofenzymeswithinthecageandentrancearerepresentedbythenumberofarrows[32],,(CPO),150400!(MCF),[33]Zhang[34],,1734nm,,,,,FSM216[35]2(PGA),[3640]2004,Chong[36]SBA215,SHC6H5CCNH2()CN(COOH)PGA,CCPGA,,PGA,,,3.2()Dave[45]2,,Cosnier[46]TiO2,TiO2,H2O2,TiO2[47],TiO2SnO2,,Dai[48](Hb)HMS,HbPHMSHbHMS,HbH2O2NO2-,014610molPLH2O2013318molPLNO2-,HMS,TiO2TiO2[49],pH7,CTiO2,C3,310-8ms-1,210-14m2s-1,Nb2O5[50,51]743110Nb2O5,(C)Nb2O5,,Nb2O5,011molPL011mmolPLH2O2,,,3.3,,,;,,Horcajada[52]MCM241,MCM241,215316nm,Vallet2Regi[53],[54]:,MCM241;,2,Zeng[55]MCM241,,;MCM241,,MCM241,,,,,2003,Fujiwara[56,57]MCM241,310nm,,250nm,,Shi[58]HMS()(3),,(layer2by2layertechnique),pH,,[59][60],,,3.4,[61,62](hydroxycarbonoapatite)250nm,,,[6366],,,843118MCM241(P2MCM241)[63]MCM24113,MCM2412,,,SBA215MCM248MCM241[64]SBA215MCM2483060,3.5,,,2Kisler[67]MCM241MCM248,Han[68]SBA215MCF,,,,Hata[69],,1018%(0178%),Lee[70]MCM248SBA215,,C18SBA215,62[71],C182SBA215,,,,Katiyar[72],SBA215[73],4,,,,,,,,,,[74],,,,,[75],,SBA215,10min8,,,,,,,,,,,,[76],943110,[1]BeckSJ,VartuliJC,RothWJ,etal.J.Am.Chem.Soc.,1992,114:1083410843[2]KresgeCT,LeonowiczME,RothWJ,etal.Nature,1992,359:710712[3](ChenFX),(HuangXD),(LiQZ).(ChineseScienceBulletin),1999,44(18):19051920[4]TaguchiA,SchthF.Micropor.Mesopor.Mater.,2005,77:145[5]TrongOnD,Desplantier2GiscardD,DanumahC,etal.Appl.Catal.A,2001,222(1P2):299357[6]VandeWaterLGA,MaschmeyerT.TopicsinCatalysis,2004,29:6777[7]CejkaJ.Appl.Catal.A,2003,254(2):327338[8]EllerbyLM,NishidaCR,NishidaF,etal.Science,1992,255(5048):11131115[9]LanEH,DunnB,ValentineJS,etal.J.Sol2GelSci.Tech.,1996,7:109116[10]MillerJM,DunnB,ValentineJS,etal.J.Non2Cryst.Solids,1996,202:279289[11]DiazJF,BalkusKJJr.J.Mol.Catal.B:Enzym.,1996,2:115126[12]Gimon2KinselME,JimenezVL,WashmonL,etal.Stud.Surf.Sci.Catal.,1998,117:373380[13]WeiY,XuJ,FengQ,etal.Mater.Lett.,2000,44:611[14]HeJ,LiXF,EvansDG,etal.J.Mol.Catal.B:Enzym.,2000,11:4553[15]TakahashiH,LiB,SasakiT,etal.Chem.Mater.,2000,12:33013305[16]Washmon2KrielL,JimenezVL,BalkusKJJr.J.Mol.Catal.B:Enzym.,2000,10:453469[17]FengX,FryxellGE,WangLQ,etal.Science,1997,276(5314):923926[18]YiuYJ,WrightPA,BottingNP,etal.J.Mol.Catal.B:Enzym.,2001,15:8192[19]GoradiaD,CooneyJ,HodnettBK,etal.J.Mol.Catal.B:Eezym.,2005,32:231239[20](ZhouCF),(ZhuJH).(JiangsuChemicalIndustry),2004,4:912[21]TakahashiH,LiB,SasakiT,etal.Micropor.Mesopor.Mater.,2001,44P45:755762[22]HernndezMCR,WejebeJEM,AlcntaraJIV,etal.Micropor.Mesopor.Mater.,2005,80:2531[23]GoradiaD,CooneyJ,HodnettBK,etal.J.Mol.Catal.B:Enzym.,2005,32:231239[24]PandyaPH,JasraRV,NewalkarBL,etal.Micropor.Mesopor.Mater.,2005,77:6777[25]JorgeA,MarcelaA,IsmaelBJ,etal.Micropor.Mesopor.Mater.,2005,83:193200[26]HanK,WuZJ,LeeJ,etal.BiochemicalEngineering,2005,22:161166[27]DeereJ,MagnerE,WallJG,etal.J.Phys.Chem.B,2002,106:73407347[28]LeiCH,ShinYS,LiuJ,etal.J.Am.Chem.Soc.,2002,124:1124211243[29]JacklerG,SteitzR,CzeslikC.Langmuir,2002,18:65656570[30]FanJ,LeiJ,ZhaoDY,etal.Chem.Commun.,2003,21402141[31]LeiJ,FanJ,ZhaoDY,etal.Micropor.Mesopor.Mater.,2004,73(3):121128[32]FanJ,YuCZ,ZhaoDY,etal.Angew.Chem.Int.Ed.,2003,42:31463150[33]HanYJ,WatsonJT,StuckyGD,etal.J.Mol.Catal.B:Enzym.,2002,17:18[34]ZhangX,GuanRF,WuDQ,etal.J.Mol.Catal.B:Enzym.,2005,33:4350[35]SasakiT,Kajin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