大气颗粒物源解析受体模型应用研究及发展现状

,(,100044):,:;;;:X823:A:100226002(2007)0120038204ResearchandDevelopmentStatusofReceptorModelonSourceApportionmentofAtmosphericParticulateMatterJINLei,etal(BeijingEnvironmentalMonitoringCentre,Beijing100044,China)Abstract:Basedonextensiveliteraturesearch,theprinciple,characteristicsandapplicationsofdifferentreceptormodelonsourceapportionmentofatmosphericparticulatematterwerecomparedandanalyzed.ThesemodelsincludedChemicalMassBalance(CMB),Improved-source-apportionmenttechnique,PrincipalFactorAnalysis(PFA)andPositiveMatrixFactorization(PMF).Thelatestdevelopmenttrendswereintroduced,suchassingleparticlesourceapportionmentbasedonprotonmicroprobe,organictracertechniqueandcombinationofdiffusionmodelandreceptormodel.Keywords:Sourceapportionment;Receptormodel;CMB;PFA:2006209213:(1979-),,,.(),,,(,1995)2070,80,,(CMB)CMB1111(CMB)(CMB),EPAPM10PPM215VOC,CMB81011111CMBCMB,,,:(1),;(2),;(3),;(4);(5);(6)11112CMBCMB,,23120072EnvironmentalMonitoringinChinaVol.23No.1Feb.2007©1994-2007ChinaAcademicJournalElectronicPublishingHouse.Allrightsreserved.(MLR),,,;;,;;,;,,,,,,(a,2000b,2000)CMB,CMB,,,,,,,(,1995),,CMB(,2000)11113CMB,CMB(,1996;,2001;,2001;,2000;,2000;,1996a,2003),CMBPM10(,1997;,1998,2003),,11114CMBCMB,,,CMB,CMB,CMB,,,,(,2002)NKCMB210,CMB710,CMB(,2002),19992000(,2003)112(FactorAnalysis,FA)11211(FA),(Blifford),,,,,,,,(,2002),,,,:39©1994-2007ChinaAcademicJournalElectronicPublishingHouse.Allrightsreserved.(,1990),,,(PFA)(PMF)(TTFA)(TRFA)11212(PFA),,,,,,,,,,,Statistica610(,2003;,2002),PM10,(b,2003)11213(PMF)PaateroTapper1993,,,,,(,2002)2000PM215,PM2156,PM215(,2002),,,;,,(,1995);B-P(PPR)(,19992000)(RS)(a,b,2003),(,20002003)2211,,,(ProtonMicroprobe,PM),Micro-PIXE(Particle-inducedX-rayEmission),,(,2004),,,,,,,,,(,2004),,,,1996(,2001)212CMBCMB,4023120072©1994-2007ChinaAcademicJournalElectronicPublishingHouse.Allrightsreserved.(Gorden,19801988),,(,2005),,Schauer2090(organictracertechnique),(OC)(Schauer,1996Cass,1998),CMB,,,PM215(,2005)213,,,,;,,,1985Chow,,,,:[1],,,.[J].,2001,22(2):51-54.[2],,.[J].,2002,23():128-130.[3],,,.[J].,2003.[4],,,.TSP[J].,2003,3(5):40-43.[5],.[J].,2002,22(4):499-502.[6],,.[J].,1997,16(10):15-17.[10],,,,,.[J].,2001,21(6):660-663.[7],,.[J].,2004,27(1):27-34.[8],.[J].,2002,24(3):55-59.[9],,.[J].,1995,15(4):252-257.[10],,.[J].,2000,22(5):58-60.[11],,.PPR[J].,2000,13(5):38-40.[12],.[J].,2003,23(1):142-144.[13].[J].,1999,19(3):270-272.[14],,.[J].,2003,35(4):112-114.[15],.[J].,2003,23(1):142-144.[16],.PM10[J].,2003,24(4):535-536.[17],.CMBTSP[J].,1996,18(1):29-38.[18],,.[J].,2001,2:46-48.[19],,,.[J].,2000,19(4):12-15.[20],,,.-TEDA[J].,1996,9(1):9-14.[21],.[J].,2000,12(4):18-21.[22],,.(TSP)[J].,2001,21(1):88-94.:41©1994-2007ChinaAcademicJournalElectronicPublishingHouse.Allrightsreserved.:([2004]186).:(1977-),,,,.[23],,.-[J].,1998,11(5):51-54.[24],,,,.[J].,2001,23(5):262-264.[25],,,.-[J].,2000,20(Suppl.):2-6.[26],,,,,.[J].,2002,23(6):11-16.[27],,.[J].,1994,7(3):1-9.[28],,.[J].,1998,18(1):62-67.[29],,,.()-[J].(,),2003.[30],,,.(II)-[J].(,),2003.[31],,,.PM215[J].,2005,18(5):1-5.[32]GordenGE.Receptormodels[J].EnvironSciTechnol,1980,14:792-8001[33]GordenGE.Receptormodels[J].EnvironSciTechnol,1988,22:1132-11421[34]SchauerJJ,RoggeWF,HildemannLM,etal.Sourceapportionmentofairborneparticulatematterusingorganiccompoundsastracers[J].AtmosEnviron,1996,30(22):3837-38551[35]CassGR.Organicmoleculartracersforparticulateairpollutionsources[J].TrendsinAnalyticalChemistry,1998,17(6):356-36611,1,1,2,1,1,1,1(1.,100029;2.,210097):MODIS,,,,;,,,,;,,20022005,:;;;;MODIS:X87:A:100226002(2007)0120042208EvaluationoftheAgriculturalResiduesBurningReductioninChinaUsingMODISFireProductHELi-ming1,etal(1.EnvironmentalSatelliteCenterPreparingOffice,StateEnvironmentalProtectionAdministration,Beijing100029,China)Abstract:Agriculturalresiduesarematerialsleftoverfromtheproductionofcrops,whichincludethestraw(orstalks)ofrice,wheat,maize,sugarcane,andcerealstrawsetc.ThetotalamountofagriculturalresiduesinChinaisabout660milliontonseveryyear,whileonethirdremainsunusedandmostlyburntdirectlyinthefield.Theburningofstrawproducesanamountofcarbondioxideandsmoke,whichconcernsovertheadversehealthandenvironmenteffect.TheAgriculturalResiduesBurningReductionAct,topreventthefarmers23120072EnvironmentalMonitoringinChinaVol.23No.1Feb.2007©1994-2007ChinaAcademicJournalElectronicPublishingHouse.Allrightsreserved.